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500 个结果
  • 简介:Carbonclothmodifiedbyhydrothermaltreatmentinammoniawaterisdevelopedasthepositiveelectrodewithhighelectrochemicalperformanceforvanadiumredoxflowbatteries.TheSEMshowsthatthetreatmenthasnoobviousinfluenceonthemorphologyofcarboncloth.XPSmeasurementsindicatethatthenitrogenousfunctionalgroupscanbeintroducedonthesurfaceofcarbonclothsuccessfully.TheelectrochemicalperformanceofV(IV)/V(V)redoxcoupleonthepreparedelectrodeisevaluatedwithcyclicvoltammetryandlinearsweepvoltammetrymeasurements.TheN-dopedcarbonclothexhibitsoutstandingelectrochemicalactivityandreversibilitytowardV(IV)/V(V)redoxcouple.TherateconstantofV(IV)/V(V)redoxreactiononcarbonclothcanincreaseto2.27×10-4cm/sfrom1.47×10-4cm/safternitrogendoping.ThecellusingN-dopedcarbonclothaspositiveelectrodehaslargerdischargecapacityandhigherenergyefficiencycomparedwiththecellusingpristinecarboncloth.TheaverageenergyefficiencyofthecellusingN-dopedcarbonclothfor50cyclesat30mA/cm2is87.8%,4.3%largerthanthatofthecellusingpristinecarboncloth.ItindicatesthattheN-dopedcarbonclothhasapromiseapplicationprospectinvanadiumredoxflowbatteries.

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  • 简介:Variousindexstructureshaverecentlybeenproposedtofacilitatehigh-dimensionalKNNqueries,amongwhichthetechniquesofapproximatevectorpresentationandone-dimensional(1D)transformationcanbreakthecurseofdimensionality.Basedonthetwotechniquesabove,anovelhigh-dimensionalindexisproposed,calledBit-codeandDistancebasedindex(BD).BDisbasedonaspecialpartitioningstrategywhichisoptimizedforhigh-dimensionaldata.Bythedefinitionsofbitcodeandtransformationfunction,ahigh-dimensionalvectorcanbefirstapproximatelyrepresentedandthentransformedintoa1Dvector,thekeymanagedbyaB+-tree.AnewKNNsearchalgorithmisalsoproposedthatexploitsthebitcodeanddistancetoprunethesearchspacemoreeffectively.ResultsofextensiveexperimentsusingbothsyntheticandrealdatademonstratedthatBDout-performstheexistingindexstructuresforKNNsearchinhigh-dimensionalspaces.

  • 标签: 高维空间 快速KNN搜索 比特码 索引结构
  • 简介:Thispaperpresentsanexperimentalstudyofthethree-dimensionalturbulentflowfieldsinalowspeedannularcascadeofhighturningangleturbineblades.Detailedmeasurementswereperformedonthebladesurfacesandmid-streamsurfaceinthepassageandatthreeaxialplanesdownstreamofthecascadebyusingwallstaticpressuretaps,afive-holeprobeandahot-wireanemometer,Thetestdataincludestaticpressuredistributiononbladesurfaces,totalpressurelosscofeeicient,meanflowvelocitycomponents.radialflowangle,turbulenceintensityandReynoldsshearstress.Analysesofthethree-dimensionalcascadeflowcharacteristicsweremadeonthenosetlocationofhighlossvortices.thevariationofpressuregradientinsidethecascadepassageandthepropertiesofendwallboundarylayerstotalpressurelossdistributions,secondaryvortexturbulentdissipationandwakedecaydowntreamofthecascade.Theseexperimentalresultsarevaluableforrevealingthedetailsofthecomplexvortexflowstructureinmodernhighlyloadedaxialturbomachinesandvalidatingthethree-dimensionalflownumericalcomputationcodes.

  • 标签: 透平机叶片 级联损耗 紊流
  • 简介:Flowbatterieswithhighenergydensityandlongcyclelifehavebeenpursuedtoadvancetheprogressofenergystorageandgridapplication.Non-aqueousbatterieswithwidevoltagewindowsrepresentapromisingtechnologywithoutthelimitationofwaterelectrolysis,buttheysufferfromlowelectrolyteconcentrationandunsatisfactorybatteryperformance.Here,anon-aqueouslithiumbrominerechargeablebatteryisproposed,whichisbasedonBr2/Br-andLi+/Liasactiveredoxpairs,withfastredoxkineticsandgoodstability.TheLi/Brbatterycombinestheadvantagesofhighoutputvoltage(3.1V),electrolyteconcentration(3.0mol/L),maximumpowerdensity(29.1mW/cm2)andpracticalenergydensity(232.6Wh/kg).Additionally,thebatterydisplaysacolumbicefficiency(CE)of90.0%,avoltageefficiency(VE)of88.0%andanenergyefficiency(EE)of80.0%at1.0mA/cm2aftercontinuouslyrunningformorethan1000cycles,whichisbyfarthelongestcyclelifereportedfornon-aqueousflowbatteries.

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  • 简介:Weinvestigatethediffractionoftheguidedmodesofadielectricslabwaveguideonasimpleintegratedstructureconsistingofasingledielectricridgeonthesurfaceofthewaveguide.Numericalsimulationsbasedonaperiodicrigorouscoupled-waveanalysisdemonstratetheexistenceofsharpresonantfeaturesandboundstatesinthecontinuum(BICs)inthereflectanceandtransmittancespectraoccurringattheobliqueincidenceofatransverseelectric(TE)-polarizedguidedmodeontheridge.Usingtheeffectiveindexmethod,weexplaintheresonancesbytheexcitationofcross-polarizedmodesoftheridge.FormationoftheBICsareconfirmedusingatheoreticalmodelbasedoncoupled-wavetheory.ThemodelsuggeststhattheBICsoccurduetothecouplingofquasi-TEandquasi-transverse-magneticmodesofthestructure.SimpleanalyticalexpressionsfortheangleofincidenceandtheridgewidthpredictingthelocationoftheBICsareobtained.Theexistenceofhigh-QresonancesandBICsenablesusingtheconsideredintegratedstructureforsensing,transformationofopticalsignals,andenhancingnonlinearlight–matterinteractions.DuetotheLorentzianlineshapeoftheresonancesneartheBICs,thestructureisalsopromisingforfilteringapplications.

  • 标签: Bound states HIGH-Q RESONANCES SLAB waveguide
  • 简介:快打扫方法的高顺序最近在文学被开发了高效地解决静态的Hamilton-Jacobi方程。与快打扫方法的第一份订单作比较,快大规模的高顺序方法是更精确的,但是因为精确地在流入边界附近对待点是特别地重要的更宽的数字模板,他们经常在边界附近为几个格子点要求另外的数字边界处理,当信息将流进计算领域并且将影响全球精确性。在文学,在这些边界点的数字答案也与准确答案被修理,它不总是是可行的,或与第一顺序discretization计算了,它能减少全球精确性。在这篇论文,我们讨论二策略处理流入边界条件。一个人基于快在边界和理查森推测附近与几种不同网孔尺寸打扫方法的第一份订单的数字答案,其它基于一个Lax-Wendroff类型过程到反复利用PDE以正切的衍生物给正常写空间衍生物到流入边界,从而在格子获得高顺序解决方案值指在流入边界附近。我们用快大规模高度探索这二条途径顺序WENO计划在[18]为作为一个代表性的例子解决静态的Eikonal方程。数字例子被给表明这二条途径的表演。

  • 标签: 数字 边界条件 短时距方程 计算方法
  • 简介:Combustioncharacteristicsofmethanejetflamesinanindustrialburnerworkinginhightemperaturecombustionregimewereinvestigatedexperimentallyandnumericallytoclarifytheeffectsofswirlinghightemperatureaironcombustion.Speziale-Sarkar-Gatski(SSG)Reynoldsstressmodel,Eddy-DissipationModel(EDM),DiscreteOrdinatesMethod(DTM)combinedwithWeighted-Sum-of-GreyGasesModel(WSGG)wereemployedforthenumericalsimulation.BothThermal-NOandPrompt-NOmechanismwereconsideredtoevaluatetheNOformation.Temperaturedistribution,NOemissionsbyexperimentandcomputationinswirlingandnon-swirlingpatternsshowcombustioncharacteristicsofmethanejetflamesaretotallydifferent.Non-swirlinghightemperatureairmadehighNOformationwhilesignificantNOprohibitionwereachievedbyswirlinghightemperatureair.Furthermore,velocityfields,dimensionlessmajorspeciesmolefractiondistributionsandThermal-NOmolarreactionrateprofilesbycomputationinterpretaninnerexhaustgasrecirculationformedinthecombustionzoneinswirlingcase.

  • 标签: 高温空气燃烧 NO生成 燃烧特性 旋流式 甲烷 雷诺应力模型
  • 简介:Wereportonasystematicexperimentalstudyonthefluorescencespectraproducedfromafemtosecondlaserfilamentinairunderahighelectricfield.Theelectricfieldalonewasstrongenoughtocreatecoronadischarge(CD).Fluorescencespectrafromneutralandionicairmoleculesweremeasuredandcomparedwithpurehigh-voltageCDandpurelaserfilamentation(FIL).Amongthem,highelectricfieldassistedlaserFILproducednitrogenfluorescencemoreefficientlythaneitherpureCDorpureFILprocesses.Thenonlinearenhancementoffluorescencefromtheinteractionofthelaserfilamentandcoronadischargingelectricfieldresultedinamoreefficientionizationalongthelaserfilamentzone,whichwasconfirmedbythespectroscopicmeasurementofbothionization-inducedfluorescenceandplasma-scattered800nmlaserpulses.Thisisbelievedtobethekeyprecursorprocessforfilament-guideddischarge.

  • 标签: FEMTOSECOND LASER FILAMENTATION FILAMENT induced fluorescence
  • 简介:ErrorestimatesofGalerkinmethodforKuramoto-Sivashingsky(K-S)equationinspacedimension≥3arederivedinthepaper.Theseresultsfurnishstrongevidenceforthecom-putationofthesolutions.

  • 标签: K-S equation GALERKIN method ERROR estimate.
  • 简介:Thispaperdescribesanoverviewofourrecentdiscovery–cleardemonstrationthatLiFcrystalscanbeefficientlyusedasahigh-performanceneutronimagingdetectorbasedonopticallystimulatedluminescenceofcolorcentersgeneratedbyneutronirradiation.Itisshownthattheneutronimageswehaveobtainedarealmostfreefromgranularnoise,haveaspatialresolutionof~5.4μmandalinearresponsewithadynamicrangeofatleast103.ThehighcontrastandgoodsensitivityofLiFcrystalsallowustodistinguishtwoholeswithlessthan2%transmittancedifference.Weproposetousesuchdetectorsinareaswherehighspatialresolutionwithhighimagegradationresolutionisneeded,includingdiagnosticsofdifferentplasmasourcessuchaslaserandz-pinchproducedplasmas.

  • 标签: color CENTERS Li F CRYSTALS NEUTRON
  • 简介:Inthepreviouspapers,ahighperformancesparsestaticsolverwithtwo-levelunrollingbasedonacell-sparsestorageschemewasreported.Althoughthesolverreachesquiteahighefficiencyforabigpercentageoffiniteelementanalysisbenchmarktests,theMFLOPS(millionfloatingoperationspersecond)ofLDLTfactorizationofbenchmarktestsvaryonaDellPentiumⅣ850MHzmachinefrom100to456dependingontheaveragesizeofthesuper-equations,i.e.,ontheaveragedepthofunrolling.Inthispaper,anewsparsestaticsolverwithtwo-levelunrollingthatemploystheconceptofmaster-equationsandsearchesforanappropriatedepthsofunrollingisproposed.ThenewsolverprovideshigherMFLOPSforLDLTfactorizationofbenchmarktests,andthereforespeedsupthesolutionprocess.

  • 标签: 高性能计算机 稀疏矩阵 有限元分析 存储设备 逻辑运算
  • 简介:Afiniteelementisestablishedforanalyzingthedynamicalmechanicsanddeformationofsteelframeathightemperaturewhenitisrapidlycooleddownbyspraywaterinfirefighting.Thesimulationresultshowsthatremarkablemechanicalcouplingeffectsareproducedintheprocess,andthesectionalstressinrapidcoolingdownisfoundconsiderablylargerthanthatinheating-up.Meanwhile,thestressanddeformationofabeammainlyrelatedtocoolingrateandlocationaremuchlargerthanthoseofacolumninrapidcooling.Infirefighting,thestructureonthefirstorsecondfloorwasmoredangerousthanthoseonotherfloorsinrapidcooling.Theseresultscouldprovideatheoreticalreferenceforthedesignofsteelstructureandfirefighting.

  • 标签: 快速冷却 动态力学 钢框架 变形 喷水灭火 高温
  • 简介:Inthiswork,viaafacilesolvothermalroute,wesynthesizedananodematerialforlithiumionbatteries(LIBs)—SnS_2nanoparticle/graphene(SnS_2NP/GNs)nanocomposite.ThenanocompositeconsistsofSnS_2nanoparticleswithanaveragediameterof4nmandgraphenenanosheetswithoutrestacking.TheSnS_2nanoparticlesarefirmlyanchoredonthegraphenenanosheets.AsananodematerialforLIBs,thenanocompositeexhibitsgoodListorageperformanceespeciallyhighrateperformance.Atthehighcurrentrateof5,10,and20A/g,thenanocompositedeliveredhighcapacitiesof525,443,and378mAh/g,respectively.ThegoodconductivityofthegraphenenanosheetsandthesmallparticlesizeofSnS_2contributetotheelectrochemicalperformanceofSnS_2NP/GNs.

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  • 简介:TwoEu(Ⅲ)complexes,(tris-4,4,4-trifluoro-1-phenyl-1,3-butanedione)(1,10-phenanthroline)europium(Ⅲ)[Eu(tpb-H)3(phen)]and(tris-4,4,4-trifluoro-1-phenyl-1,3-butanedione)(2,2'-bipyridine)europium(Ⅲ)[Eu(tpb-H)3(bipy)]weresynthesizedfrombi-dentaloxygenandnitrogenligands.LuminescentpolymerswerefabricatedbyincorporatingdeuteratedEu(Ⅲ)complexesinpoly(methylmethacrylate)(PMMA)matrixes.LuminescentPMMAcontainingEu(tpb-D)3(phen)exhibitedrelativelyhigherquantumyield[Φ,(48.7±4)%],fasterradiationrate(kr,7.49×102s-1),sharperredemission[fullwidthathalfmaximum(FWHM),6.3nm]andlargerstimulatedemissioncross-section(SEC,1.29×10-20cm2).ThevalueofSECisthesameorderasthatofNd-glasslaserforpracticaluse.Additionally,thethermalpropertiesofEu(tpb-H)3(phen),Eu(tpb-H)3(bipy),Eu(tpb-D)3(phen)-PMMA,andEu(tpb-H)3(bipy)PMMAwerestudied,indicatingthattheEu(Ⅲ)complexesandluminescentPMMAcanbeusedforalong-termperiodinhightemperatureenvironment.PreparedluminescentpolymersincludingEu(tpb-D)3(phen)havepromisingapplicationsinnovelorganicEu(Ⅲ)devices,suchasthehigh-powerlasermaterialsandopticalfibers.

  • 标签: 聚甲基丙烯酸甲酯 发光量子效率 复合掺杂 辐射率 受激发射截面
  • 简介:Theworkpresentedinthispaperisastudyofoutputtemporalcontrastdegradationbynear-fieldqualitydeterioration,suchasintensitymodulationandwavefrontdeviation,inalargeaperturehighpowershortpulselasersystem.AtwostepfocusingalgorithmwithacoordinatetransformbasedontheFresnelapproximationinthespacedomainisusedforsimulatingtheoutputfocusedbyanoff-axisparabolicmirror.Thetemporalcontrastdegradationbyintensitymodulationandwavefrontdeviationisanalyzedandtheinfluenceofthediameteronthetemporalcontrastdegradationisrevealed.ThesimulationandassumptionresultsbasedontheparametersoftheShenGuang-IIlasersystemarecomparedwiththeonlineexperimentaltemporalcontrastdata.Thenear-fieldqualitydeteriorationmightleadtotemporalcontrastdegradation,hinderinghighertemporalcontrastinlargeaperturehighpowershortpulselasersystems.

  • 标签: FILL factor of laser beam temporal
  • 简介:Weexperimentallydemonstratehighopticalqualityfactorsilicamicrodiskresonatorsonasiliconchipwithlargewedgeanglesbyreactiveionetching.For2-μm-thickmicroresonators,wehaveachievedwedgeanglesof59°,63°,70°,and79°withopticalqualityfactorsof2.4×10~7,8.1×10~6,5.9×10~6,and7.4×10~6,respectively,from~80μmdiametermicroresonatorsinthe1550nmwavelengthband.Also,for1-μm-thickmicroresonators,wehaveobtainedanopticalqualityfactorof7.3×10~6withawedgeangleof74°.

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