A new approach to spatial source apportionment of haze pollution in large scale and its application in China

(整期优先)网络出版时间:2018-02-12
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Long-lastingexpansionofhazepollutioninChinahasalreadypresentedasternchallengetoregionaljointpreventionandcontrol.Thereisanurgentneedtoenlargeandreconstructthecoverageofjointpreventionandcontrolofairpollutioninkeyarea.Airqualitymodelscanidentifyandquantifytheregionalcontributionofhazepollutionanditskeycomponentswiththehelpofnumericalsimulation,butitisdifficulttobeappliedtolargerspatialscaleduetothecomplexityofmodelparameters.Thetimeseriesanalysiscanrecognizetheexistenceofspatialinteractionofhazepollutionbetweencities,butithasnotyetbeenusedtofurtheridentifythespatialsourcesofhazepollutioninlargescale.Usingeconometricframeworkoftimeseriesanalysis,thispaperdevelopedanewapproachtoperformspatialsourceapportionment.WeappliedthisapproachtocalculatethecontributionfromspatialsourcesofhazepollutioninChina,usingthemonitoringdataofparticulatematter(PM2.5)across161Chinesecities.Thisapproachovercamethelimitationofnumericalsimulationthatthemodelcomplexityincreasesatexcesswiththeexpansionofsamplerange,andcouldeffectivelydealwithseverelarge-scalehazeepisodes.